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Greycap is a poison made from a toadstool.[1]

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A Clash of Kings

Tyrion Lannister sees powdered greycap in Grand Maester Pycelle's collection of medicines and poisons.[2]

A Storm of Swords

During Tyrion Lannister's trial for the death of King Joffrey I Baratheon, Pycelle claims that Tyrion stole a sample of greycap as well as other drugs from Pycelle's collection.[1]